高雄位於南台灣，是個高度密集的工業地區，在懸浮微粒及戴奧辛(PCDDs)和呋喃(PCDFs)的貢獻上較其他地區顯著。近年來，台灣對於空氣汙染、土壤危害及食品安全的議題上越來越重視，因此研究此類有毒化合物的宿命是極為重要的。本研究透過戴奧辛類化合物及懸浮微粒的濃度做迴歸分析，模擬2014及2015年戴奧辛類化合物在高雄地區中小港(重工業地區)、高雄(都市地區)、美濃(鄉村地區)大氣中之乾、濕沉降通量及氣固相比例，並模擬其在每公升雨量中的濃度，分別以質量及毒性當量濃度表示之。
在本研究探討的三個地區中，其年平均細懸浮微粒濃度介於23 - 31 μg m-3，皆超過台灣之空氣品質標準。透過模式模擬之結果，高雄地區在2014年戴奧辛/呋喃的毒性當量濃度介於0.021 - 0.077 pg WHO2005-TEQ m-3 且於2015年介於0.021 - 0.072 pg WHO2005-TEQ m-3，其年平均分別為0.048 和 0.044 pg WHO2005-TEQ m-3，模擬之總沉降通量(乾沉降+濕沉降)於2014期間介於75.0 - 554.8 pg WHO2005-TEQ m-2 month-1 且在2015年時介於 46.4 - 404.3 pg WHO2005-TEQ m-2 month-1。以毒性當量觀點觀之，戴奧辛/呋喃類化合物以1,2,3,7,8-PeCCD 及 2,3,4,7,8-PeCDF對大氣中毒性貢獻量最為顯著。相較於其他兩地區，重工業之小港地區有著最高的細懸浮微粒濃度以及總沉降通量，而鄉村之美濃地區則為最少量。
在每公升雨量的戴奧辛/呋喃毒性當量方面上，高雄地區在2014年之年平均雨量中戴奧辛/呋喃濃度為0.795 pg WHO2005-TEQ L-1，且於2015年時為0.689 pg WHO2005-TEQ L-1。如同上面所述，大氣中含較多戴奧辛/呋喃濃度之小港地區雨量擁有著較高的毒性，而美濃地區則相對較低。
此研究所提供的資訊可供未來研究及擬定環境控制策略所參照，所模擬之毒性總量可做為後續排放法規之訂定及修正。

Kaohsiung in southern Taiwan has both highly industrial and rural areas, causing significantly higher concentrations of particulate matter as well as Polychlorinated dibenzo-p-dioxins (PCDDs) and polychlorinated dibenzofurans (PCDFs). In this study, the characteristics of PCDD/Fs in the ambient air of Kaohsiung (urban), Meinong (rural area) and Xiaogang (heavy industrial zone) in 2014 and 2015 were modeled based on the regression of collected PCDD/F concentrations versus the measured ambient air concentrations of PM2.5, PM10 and TSP. Further simulations for gas-particle partition, dry and wet deposition modeling will also be included in this study.
The annually average PM2.5 concentrations in the ambient air of the three areas were in the range of 23 to 31 μg m-3, all above the National Air Quality Standard of Taiwan. The simulated average concentrations of PCDD/Fs in Kaohsiung area in terms of toxicity equivalent were in the range of 0.021 - 0.077 and 0.021 - 0.072 pg WHO2005-TEQ m-3 during 2014 and 2015 and averaged 0.048 and 0.044 pg WHO2005-TEQ m-3, respectively. The average total deposition fluxes of total-PCDD/Fs-WHO2005-TEQ ranged between 75.0 - 554.8 and 46.4 - 404.3 pg WHO2005-TEQ m-2 month-1 during 2014 and 2015, with 1,2,3,7,8-PeCCD and 2,3,4,7,8-PeCDF being the dominant congeners in terms of PCDD/Fs WHO2005-TEQ. Xiaogang area with highly industrial activities had the highest concentrations of PM2.5 and PCDD/Fs and corresponding total deposition fluxes, while the Meinong in the rural site recorded the lowest.
As for the concentrations of PCDD/Fs in the raindrop, Kaohsiung has the annual concentrations in the rainfall of 0.795 and 0.689 pg WHO2005-TEQ L-1 for 2014 and 2015, respectively and averaged 0.742 pg WHO2005-TEQ L-1. Likewise, Xiaogang area with the highest concentrations of PCDD/Fs resulted in the largest value of concentration on the raindrop, while the Meinong with lower one gained the lowest.
The information provided in this work is useful for both further study and environmental control strategies, and data of emission inventory of PCDD/Fs is useful for setting up regulations of emission.

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