矽酸鹽化學風化過程中會消耗大氣中的二氧化碳，是調節長期地球氣候的重要反應，因此了解矽酸鹽化學風化是重要的課題。土壤為關鍵帶(Critical Zone)中重要的反應區，孔隙中的土壤水會和矽酸鹽進行水岩反應，因此水的化學組成可提供來自這些水/岩反應的訊息，許多前人研究也指出世界上主要河流中的同位素組成受到風化層中水岩反應有一定程度之影響。在矽酸鹽中，鋰(Lithium)是一易遷移元素，其同位素組成可作為了解矽酸鹽水岩反應及次生礦物形成過程的指標。台灣位於東亞季風帶上，秋冬之際盛行東北季風，此時也將亞洲沙塵(Asian dust)從黃土高原等經由季風帶至台灣，並透過降雨使其從大氣進入地表中。本研究針對觀雲山莊周遭的雨水及九個土壤水採樣點進行採樣，分別以ICP-OES、ICP-QMS及MC-ICP-MS分析樣品的主要元素、微量元素以及鋰同位素值(δ7Li)。
根據觀雲的雨量、雨水及土壤水的化學及鋰同位素組成，可得知雨量多寡與雨水的鋰濃度呈負相關，與雨水的δ7Li及土壤水的鋰濃度及δ7Li則無明顯相關性，且因土壤剖面淺層之黏土礦物溶解的影響使得位於15公分處之土壤水樣品無法明顯區分乾濕季樣品的差異。雨水的來源除與代表地緣關係的平均上部大陸地殼(upper continental crust, UCC)值有關外，透過東北季風輸送而來的黃土沙塵也有一定的貢獻。觀雲土壤水的鋰濃度及鋰同位素與前人文獻比較後，除了顯示出不同地點的化學差異外，採樣方法亦可能造成土壤水之鋰化學及同位素組成不同。從土壤水的Li/Na比與鋰同位素組成的關係可知觀雲地區無明顯次生礦物分化情形，並因其位於表層而以黏土礦物溶解為主要過程。

Silicate weathering is a crucial component of long-term evolution of climate through the consumption of atmospheric CO2. Soil where the water-rock between take place is an important reactive part in the critical zone. Lots previous studies show that isotopic compositions in river water around world has been affected by these Water-Rock reactions in the weathering zone. Lithium, a mobile minor element in silicate, is often used to understand the reactions of silicate and the processes of secondary minerals formations. Taiwan is located at East Asia monsoon zone. Therefore, aeolian dust of Loess Plateau is blown to Taiwan by northeast monsoon. In this study, we collected the rainwater and nine soil water samples at Kuan-Yun region. The compositions of major elements, trace elements and δ7Li of these samples were determined by ICP-OES, ICP-QMS and MC-ICP-MS respectively.
A negative correlation between rainfall and Li compositions (elemental and isotopic) in the rainwater was observed. On the contrary, no correlation was shown in soil water samples. Apart from upper continental crust (UCC), the results indicated aeolian dust from Loess Plateau play a significant role on chemical and isotopic compositions of rainwater. These suggest that Li isotope composition of our soil water is mainly controlled by the dissolution of the silicate. Unlike other similar Li isotope studies in critical zone, Kuan-Yun soil water sample have relatively low δ7Li variations and no Li isotope fractionation caused by secondary phase was noticed. This could be contributed by the differences of soil composition and short soil water residence time at Kuan-Yuan area.

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