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研究生: 張學文
Jhang, Shiao-Wun
論文名稱: 價鍵漲落系統CeMn2Si2的異常現象
Anomalous behaviors of the valence fluctuation system CeMn2Si2
指導教授: 田聰
Tien, Chen
學位類別: 碩士
Master
系所名稱: 理學院 - 物理學系
Department of Physics
論文出版年: 2010
畢業學年度: 98
語文別: 中文
論文頁數: 61
中文關鍵詞: 價鍵漲落磁阻自旋玻璃
外文關鍵詞: valence fluctuation, magnetoresistance, spin glass
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  • 本實驗是對混和價鍵系統CeMn2Si2-like (CeMn2.16Si1.84)做電性、磁性和熱性磁的研究, 我們可以在樣品CeMn2.16Si1.84上發現,當樣品放在外加高磁場(H=120 kOe)且低溫的環境下,會產生一個異常大的正磁阻,而樣品溫度在21K時,其磁阻產生高達548%的最大值,且當溫度低於21K時,磁阻值會隨著溫度的下降而變小。在磁性測量方面,當在外加低磁場(H < 100 Oe)下,樣品CeMn2.16Si1.84的溫度低於240K時,我們可以觀察到產生熱磁不可逆(thermomagnetic irreversibility,TMI)的現象,隨著外加磁場的增加,使的TMI效應慢慢變小且消失。在外加高磁場的環境下,因為樣品CeMn2.16Si1.84為混和價鍵系統,所以我們可以推測因為高磁場的存在,使的4f電子能階位移至費米能階附近,造成磁阻在低溫高磁場下有異常大的值存在,且樣品的TMI效應可能源自於鐵磁分量依附在反鐵磁有序結構或者自旋玻璃相。

    The electrical, magnetic and thermal properties of the valence fluctuation system CeMn2Si2-like (CeMn2.16Si1.84) were studied. In a magnetic field of 12 T, as the temperature decreases the magnetoresistance of CeMn2.16Si1.84 becomes positive and reaches an unusually large value 548% at 21 K. Whereas, below 21 K, the magnetoresistance decreases as the temperature decreased. The anomalously high magnetoresistance might arise from the shifted f-band over the Fermi level by a magnetic field. In a low magnetic field (H < 100 Oe), large thermomagnetic irreversibility (TMI) was observed below ~ 240 K. The TMI behavior decreases with the increasing H, and disappears with the H large enough. This behavior can be explained by the antiferromagnetic component pinned in the overall ferromagnetic ordering structure, or spin-glass phases.

    摘要 I Abstract II 誌謝 III 目錄 IV 表目錄 V 圖目錄 VII 第一章 緒論 1 第二章 理論介紹 4 第一節 晶格結構 4 第二節 金屬內部的電阻與比熱 4 第三節 磁性理論 7 第三章 實驗方法與儀器介紹 14 第一節 樣品製作 14 第二節 實驗測量方法與儀器介紹 17 第四章 實驗結果與討論 27 第一節 磁性量測 30 第二節 電阻量測 34 第五章 結論 59 參考文獻 60

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