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研究生： 高駿青
Annas, Fauzy
論文名稱： 氣體燃料燃燒中添加過氧化氫的分析
Analysis of Hydrogen Peroxide Addition to the Gaseous Fuel Combustion
指導教授： 林大惠
Lin, Ta-Hui
陳冠邦
Chen, Guan-Bang
學位類別： 博士
Doctor
系所名稱： 工學院 - 機械工程學系
Department of Mechanical Engineering
論文出版年： 2025
畢業學年度： 113
語文別： 英文
論文頁數： 108
中文關鍵詞： 甲烷 、一氧化碳 、氫氣 、過氧化氫 、預混燃燒 、絕熱火焰溫度 、層流火焰 速度 、熱釋放速率
外文關鍵詞： Methane, Carbon monoxide, Hydrogen, Hydrogen Peroxide, Premixed combustion, Adiabatic flame temperature, Laminar flame speed, Heat release rate
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    • 氣體燃料燃燒是氣體燃料與氧化劑之間的放熱化學反應、不同的氣體燃料具有各自的燃燒特性和操作條件。氧化劑強化策略（富氧或添加強氧化劑（過氧化氫））可以提高氣體燃料的燃燒性能。本研究旨在以富氧作為對比、了解添加過氧化氫對甲烷、一氧化碳和氫氣預混燃燒的影響。對一個自由傳播的一維火焰模型進行了數值研究、以研究添加過氧化氫對每種預混氣體燃料燃燒的影響。進行了預混甲烷火焰的錐形火焰實驗，以了解過氧化氫溶液對預混甲烷燃燒的影響。在標準條件下(298K 和大氣壓力)、透過添加少量含氫物質（甲烷、水蒸氣和氫氣）、對一氧化碳-空氣預混火焰的引發進行了額外的研究。所有數值和實驗工作均在423K(過氧化氫的沸點)和一個大氣壓力下進行。

    在數值觀測中、將過氧化氫添加到預混甲烷、一氧化碳和氫氣火焰中、結果表明、添加過氧化氫方案的層流火焰速度優於添加富氧方案。隨著氧化劑中氧氣百分比的增加、絕熱火焰溫度分佈從添加過氧化氫>富氧方案變成添加富氧方案>添加過氧化氫方案。我們將這兩種方案的交點定義為交點溫度。化學效應對層流火焰速度有顯著的貢獻、尤其是在添加較多過氧化氫的情況下。在一氧化碳-空氣燃燒的引發過程中、添加不同的含氫物種具有難以區分的絕熱火焰溫度、而添加甲烷的層流火焰速度分佈分別高於添加氫氣和水蒸氣的情況。此外、層流火焰速度與放熱速率呈正相關、添加甲烷可顯著提高放熱速率。

    實驗觀察發現、當過氧化氫濃度為60%時、層流火焰速度保持不變、而當過氧化氫濃度高於70%時、層流火焰速度增加。實驗和數值模擬一致地證明了最大層流火焰速度的混合當量比與不同過氧化氫添加量和濃度之間存在相關性。與數值模擬相比、實驗計算出的火焰速度被低估、可能是由於過氧化氫的早期分解所致。建議使用濃度高於70%的過氧化氫溶液、以提高預混甲烷/空氣火焰的整體層流火焰速度。

    Gases fuel combustion is an exothermic chemical reaction between the gaseous fuel and oxidizers,  where different gaseous fuel has their own combustion characteristics and operating conditions. An oxidizer enhancement strategy (oxygen-enrichment or adding a strong oxidant (hydrogen peroxide)) can increase the gaseous fuel combustion performance. This study aimed to understand the effects of hydrogen peroxide addition to the premixed combustion of methane, carbon monoxide, and hydrogen using oxygen enrichment as a comparison. A freely propagating one-dimensional flame model is numerically investigated to study the effects of hydrogen peroxide addition to each premixed gaseous fuel combustion. A conical flame experiment for a premixed methane flame was performed to understand the effects of hydrogen peroxide solution on the premixed methane combustion. An additional investigation on the initiation of carbon monoxide-air premixed flame was performed using a small addition of hydrogenous species (methane, water vapor, and hydrogen) at standard conditions (298K and atmospheric pressure). All the numerical and experimental works have been done at 423K (the boiling point of hydrogen peroxide) and atmospheric pressure.

    In the numerical observation, adding the hydrogen peroxide to the premixed methane, carbon monoxide, and hydrogen flame showed that the laminar flame speed of the hydrogen peroxide addition scenario dominates over the oxygen-enrichment scenario. The adiabatic flame temperature distribution changed upon hydrogen peroxide addition > oxygen-enrichment scenario to the oxygen-enrichment scenario > hydrogen peroxide addition with increasing oxygen percentage in oxidizers. We define the intersection between these two scenarios as the intersection temperature. The chemical effect has a noticeable contribution to the laminar flame speed, especially in higher hydrogen peroxide additions. In the case of the initiation of carbon monoxide-air combustion, adding different hydrogenous species has an indistinguishable adiabatic flame temperature, while adding methane has a higher laminar flame speed distribution compared with hydrogen and water steam addition, respectively. Furthermore, the laminar flame speed positively correlates with the heat release rate, and adding methane results in a noticeable increase in the heat release rate.

    In the experimental observation, the laminar flame speed remains unchanged at a hydrogen peroxide concentration of 60%, while it increases at a hydrogen peroxide concentration higher than 70%. The experiment and numerical simulation consistently correlated the mixture equivalence ratio of the maximum laminar flame speed on various hydrogen peroxide additions and concentrations. The flame speed from the experiment was underestimated compared with the numerical simulation, presumably owing to the early decomposition of hydrogen peroxide. Using a hydrogen peroxide solution with a concentration higher than 70% is advisable to increase the overall laminar flame speed of premixed methane/air flames.

    Abstract i 摘要 iii Acknowledgment v Table of Contents vii List of Figures ix List of Tables xiii Nomenclature xv Chapter 1 Introduction 1 1.1 Hydrogen peroxide (H2O2) 3 1.2 Oxidizer enhancement strategy 5 1.2.1 Oxygen enrichment combustion 5 1.2.2 Hydrogen peroxide addition 6 1.3 Common gaseous fuel combustion 7 1.3.1 Methane combustion 7 1.3.2 Carbon monoxide combustion 7 1.3.3 Hydrogen combustion 9 1.4 Motivations and objectives 10 1.5 Structure of the dissertation 11 Chapter 2 Methodology 13 2.1 Numerical methodology 13 2.1.1 Governing equation 14 2.1.2 Numerical setup 17 2.1.3 Chemical mechanism 21 2.2 Experimental methodology 22 2.2.1 Experimental set-up 22 2.2.2 Phase transition behaviour of H2O2 solutions 23 2.2.3 Evaporation system of hydrogen peroxide solution 27 2.2.4 Flame speed measurement methodology 28 2.2.5 Uncertainty analysis 30 Chapter 3 Analysis of H2O2 additions and O2 - enrichment on CH4 premixed combustion 31 3.1 Pure gaseous H2O2 addition and oxygen (O2) - enrichment premixed methane (CH4) combustion 32 3.1.1 Mechanism validation 32 3.1.2 Adiabatic flame temperature 34 3.1.3 Laminar flame speed 35 3.1.4 Heat release rate 39 3.2 Applications of the addition of H2O2 solution on CH4 premixed combustion 47 3.2.1 Experimental validation 47 3.2.2 Numerical simulations 48 3.2.3 Experimental results 51 3.2.3.1 Effect of different H2O2 additions on the SL 51 3.2.3.2 Effect of different H2O2 concentrations on the SL 53 3.2.3.3 Comparison between numerical and experimental results 54 4 Analysis of H2O2 additions and O2 - enrichment on CO premixed combustion 57 4.1 Pure gaseous H2O2 addition and O2 - enrichment premixed CO combustion 58 4.1.1 Mechanism validation 58 4.1.2 Laminar flame speed 60 4.1.3 Adiabatic flame temperature 61 4.2 Initiation of the CO/air premixed flame 61 4.2.1 Effects of different hydrogenous species additions on the Tad and SoL 62 4.2.2 Effects of different hydrogenous species additions on HRR 67 Chapter 5 Analysis of pure gaseous H2O2 additions and O2 - enrichment on H2 premixed combustion 71 5.1 Mechanism validation 71 5.2 Laminar flame speed 73 5.3 Adiabatic flame temperature 74 Chapter 6 General comparison 75 6.1 General comparison 75 Chapter 7 Conclusions and future works 79 7.1 Conclusions 79 7.2 Future works 81 References 83 List of Publications 89

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