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研究生: 陳翊婷
Chen, Yi-Ting
論文名稱: 探討TI/YIG雙層薄膜之自旋幫浦效應研究
Study the effect of spin pumping in the TI/YIG bilayer system
指導教授: 黃榮俊
Huang, J.C.A.
學位類別: 碩士
Master
系所名稱: 理學院 - 物理學系
Department of Physics
論文出版年: 2016
畢業學年度: 104
語文別: 中文
論文頁數: 62
中文關鍵詞: 自旋幫浦拓樸絕緣體
外文關鍵詞: YIG, Bi2Se3, spin pumping, topological insulators
相關次數: 點閱:76下載:4
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  •   本實驗中採用雙層薄膜Bi2Se3/YIG的結構,研究以拓樸絕緣體Bi2Se3作為自旋流偵測層,並量測spin pumping的實驗。
      首先成長出良好結構及磁性的磁性絕緣層YIG,再於上方成長最佳化成長參數後的Bi2Se3層,以自旋幫浦電壓訊號、電性及薄膜結構作為參數調整之依據,並量測其自旋幫浦的電壓訊號。而後進行固定YIG厚度並改變Bi2Se3層厚度,觀察電壓訊號的變化,並選取訊號較明顯且轉換效率亦高的Bi2Se3厚度作Sb(Antimony)的摻雜變化,在本實驗中是選定12nm的Bi2Se3做摻雜。
      在變化Sb摻雜量的自旋幫浦量測中,觀察隨摻雜量而改變的電壓訊號,並推測可能影響原因來自電阻值變化、界面處差異性、載子濃度改變、摻雜的取代機制等等。於本實驗中推測,其中最主要影響機制應為摻雜對電阻值的影響及摻雜的取代行為影響了整體的SOC強度,並以此說明為何摻雜後電壓訊號會上升及自旋流與電流間轉換效率會隨摻雜量增加而下降的現象。

    Spin pumping is a mechanism that generates spin currents from ferromagnetic metal (FM) and injects into normal metal (NM), while we can detect ISHE voltage signal in the NM layer. We choose Y3Fe5O12 (YIG) grown on Gd3Ga5O12 (GGG) as ferromagnetic metal insulator (FMI) layer, and Bismuth Selenide (Bi2Se3) as NM layer which transfers pure spin current into charge current. We changed the thickness of Bi2Se3 in this experiment, and choose the appropriate thickness to adulterate Antimony (Sb), while doping Sb is used as decreasing the carrier concentration and increasing the thin film resistance in Bi2Se3. We observed the changing of spin pumping voltage signal after doping Sb, and discussed the origin of changing in spin pumping signal.
    In our experiment, we observed two results after doping Sb in Bi2Se3, for one thing, the spin pumping voltage has increased, and for another thing, the spin current conversion efficiency has decreased. This consequence might come from the changing of film resistance and Sb substituting in Bi site.
    After all, we get high spin current conversion efficiency in Bi2Se3 system, and get high spin current detection efficiency in Sb-doped Bi2Se3 system. This experiment shows that topological insulators with strong spin-orbit coupling could be used in spintronic devices at room temperature.

    目錄 摘要 I Abstract II 誌謝 IX 圖目錄 XII 表目錄 XIV 第一章、緒論 1 1-1 前言 1 1-2 文獻回顧 2 1-3 研究動機 13 第二章、相關理論介紹 16 2-1 鐵磁共振(Ferromagnetic resonance, FMR) 16 2-2 自旋霍爾效應(Spin Hall Effect, SHE)及反轉自旋霍爾效應(Inverse Spin Hall Effect, ISHE) 19 2-3 自旋動量鎖定(Spin momentum locking) 20 2-4 自旋幫浦機制(Spin pumping mechanism) 21 第三章、儀器介紹與實驗步驟 23 3-1 實驗流程 23 3-2 製程樣品之儀器介紹 25 3-2-1 脈衝雷射沉積儀(Pulsed Laser Deposition, PLD) 25 3-2-2 分子束磊晶系統(Molecular Beam Epitaxy, MBE) 26 3-3 量測樣品之儀器介紹 29 3-3-1 自旋幫浦量測系統介紹 29 3-3-2 電性量測 31 3-4 分析樣品之儀器 33 3-4-1 反射式高能電子繞射儀(Reflection High Energy Electron Diffraction ,RHEED) 33 3-4-2 X光繞射儀(X-ray Diffraction, XRD) 35 3-4-3 原子力顯微鏡(Atomic Force Microscopy, AFM) 36 第四章、實驗結果與討論 39 4-1 YIG薄膜成長 39 4-1-1 YIG結構確認 39 4-1-2 YIG磁性確認 41 4-2 Bi2Se3/YIG雙層薄膜成長 44 4-2-1 Bi2Se3/YIG不同製程間量測訊號比較 44 4-2-2 Bi2Se3/YIG結構確認 45 4-3 Bi2Se3/YIG自旋幫浦量測 48 4-4 Sb-doped Bi2Se3/YIG自旋幫浦量測 51 4-5 Sb摻雜量對電壓訊號變化 55 第五章、結論 61 引用文獻 62

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