移動性污染源排放PCDD/Fs對於國內PCDD/Fs之貢獻量影響日益顯著，為瞭解移動性污染源排放PCDD/Fs之特徵，本研究針對50輛汽油SUV車、15輛柴油小客車、2輛重型柴油車及10輛機械腳踏車，進行PCDD/Fs排放之研究，藉由行車型態測試進行排氣PCDD/Fs檢測分析，以建立國內移動性污染源PCDD/Fs之排放廢氣特徵剖面，另外，將其排放廢氣之PCDD/Fs進行氣相及固相分析，並將結果與國內外相關研究文獻比較，提供國內後續進行管制移動性污染源排放PCDD/Fs之參考。
本研究車輛排放廢氣中PCDD/Fs之濃度，其範圍介於0.00943~0.234 ng I-TEQ/Nm3之間，其中SUV車、柴小客車、重型柴油車及機械腳踏車排放廢氣中之PCDD/Fs平均濃度分別為0.0553、0.0417、0.145及0.0591 ng I-TEQ/Nm3；車輛PCDD/Fs排放係數其範圍介於0.0267~2.91 ng I-TEQ/km之間，SUV車、柴小客車、重型柴油車及機械腳踏車之排放係數分別為0.113、0.105、1.86及0.0831 ng I-TEQ/km。
4種車款PCDD/Fs固相之I-TEQ毒性百分比分別為：SUV車之74.4%；柴油小客車之91.8%；重型柴油車之70.2%；機械腳踏車之85.1%， 4種車款固相I-TEQ毒性百分比平均為79.8%，即各車款排放廢氣之PCDD/Fs均以固相較具優勢，因此降低車輛粒狀物之排放，可有效管制車輛排放戴奧辛。
本研究為瞭解新舊機油對於移動性污染源排放PCDD/Fs之影響，選取L與N 兩車款機械腳踏車分別使用舊機油與新機油進行排放測試，發現固相PCDD/Fs總I-TEQ濃度，分別減少38.2%(0.0445降低至0.0275 ng I-TEQ/Nm3) 及58.2%(從0.0631降低至0.0264 ng I-TEQ/Nm3) ，總I-TEQ排放係數亦分別減少53.5%(0.141降低至0.0655 ng I-TEQ/km)及56.6%(0.105 降低至0.0456 ng I-TEQ/km)，其固相PCDD/Fs之I-TEQ濃度及排放係數均有明顯下降之趨勢，故更換新機油，應有助於減少固相PCDD/Fs之生成。
為瞭解移動性污染源排放對周界大氣之影響，進行焚化廠周界大氣採樣，結果顯示M廠大氣PCDD/Fs總I-TEQ平均濃度為0.0418 pg I-TEQ/Nm3，將M廠之各採樣點周界大氣PCDD/Fs特徵剖面與其煙道廢氣PCDD/Fs特徵剖面及分汽油休旅車、柴油小客車、重型柴油車之特徵剖面進行主要成分分析，結果顯示M廠周界大氣與其煙道廢氣之PCDD/Fs之特徵剖面並無明顯關聯性，而與汽油休旅車、柴油小客車、重型柴油車排放廢氣之PCDD/Fs特徵剖面相近，推測其周界大氣PCDD/Fs之濃度應受到周界移動污染源影響。

For these years, mobile pollution emission sources have contributed more and more in domestic polychlorinated dibenzo-p-dioxins and polychlorinated dibenzofurans (PCDD/Fs), This study examined the characteristics of polychlorinated dibenzo-p-dioxins and polychlorinated dibenzofurans (PCDD/Fs) in the exhaust gases of mobile sources. In this study, 50 vehicles of petrol SUV car, 15 vehicles of diesel oil limousine, 2 heavy-duty diesel vehicles and 10 motorcycles were investigated.
The PCDD/Fs emission factors of mobile sources were determined‚ and the overall emission quantity of PCDD/Fs from the domestic mobile sources was estimated. Finally, the influence of these emission sources on the surrounding environment was assessed.
The total PCDD/F concentrations exhaust from SUV, diesel vehicles, heavy-duty diesel vehicles and motorcycles are 0.0553, 0.0417, 0.145 and 0.0591 ng I-TEQ/Nm3, respectively. The PCDD/F emission factors from SUV, diesel vehicles, heavy-duty diesel vehicles and motorcycles are 0.113, 0.105, 1.86 and 0.0831 ng I-TEQ/km, respectively.
The particulate-phase of PCDD/Fs in the exhaust gases of SUV, diesel vehicles, heavy-duty diesel vehicles and motorcycles are 74.4%, 91.8%, 70.2% and 85.1%, respectively. Moreover, the mean I-TEQ concentration in particulate-phase is 79.8%. Due to the relatively high fraction of PCDD/Fs in particulate-phase, the PCDD/Fs emission can be effectively controlled by reducing the emission of particle in the exhaust gases of vehicles.
After using new engine oil old engine oil, the PCDD/Fs concentrations in particulate-phase were reduced 38.2% (from 0.0445 to 0.0275 ng I-TEQ/Nm3) and 58.2%(from 0.0631 to 0.0264 ng I-TEQ/Nm3), respectively, for L type and N type mechanical bicycles.
The emission factors of PCDD/F I-TEQ were also reduced 53.5% (from 0.141 to 0.0655 ng I-TEQ/km) and 56.6% (from 0.105 to 0.0456 ng I-TEQ/km), respectively, for L type and N type mechanical bicycles.
The trend of PCDD/F concentrations and I-TEQ emission factors indicated that using the new engine oil can reduce the PCDD/Fs emission of vehicles.
The research result shows the average PCDD/Fs concentrations in ambient air nearby M site (municipal solid waste incinerators [MSWIs]) is 0.0418 pg I-TEQ/Nm3, we compared cross-section of above PCDD/Fs with that inside the incinerator tunnels and SUV, diesel vehicles, heavy-duty diesel vehicles and motorcycles and found that there is no prominent relationship between cross-section characteristics of PCDD/Fs around the incinerators and inside their tunnels but cross-section characteristics of PCDD/Fs around the incinerators are so similar to out test vehicles. Therefore, we predict concentration of PCDD/Fs n ambient air nearby incinerators should be affected by mobile pollution emission sources which nearby them.

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