爲了瞭解Y工業區PCDD/Fs污染源對周遭環境之影響，本研究選定Y工業區中二座大型都市垃圾焚化爐、一座中小型廢棄物焚化爐、二座事業廢棄物焚化爐、一座醫療廢棄物焚化爐、五座電弧爐、四座煉鋼廠SINTER製程、一座煉焦爐、一座水泥窯、二座二次鋁精煉廠及一座二次銅精煉廠進行PCDD/Fs排放之研究，藉由煙道廢氣PCDD/Fs之檢測，以建立本土PCDD/Fs排放源之貢獻量及其煙道廢氣特徵剖面，並於Y工業區附近周界及非工業區周界選定十個採樣點進行採樣，調查Y工業區及非工業區周界環境中各介質（大氣、植物、土壤）之PCDD/Fs含量，藉由本研究中各類污染源之分佈及排放特性，與周界環境中PCDD/Fs 之流佈相比對，亦利用主成分分析及階層集群分析等方法分析，以釐清當地PCDD/Fs污染源污染對周遭環境之影響。研究成果如下：大型都市垃圾焚化爐、中小型廢棄物焚化爐、事業廢棄物焚化爐、醫療廢棄物焚化爐、電弧爐、煉鋼廠SINTER製程、煉焦爐、水泥窯、二次鋁精煉廠及二次銅精煉廠煙道廢氣中總PCDD/Fs I-TEQ濃度平均值分別為0.0632、0.239、0.145、1.64、0.477、0.326、0.00870、0.0138、0.0504及0.310 ng I-TEQ/Nm3；大型都市垃圾焚化爐、中小型廢棄物焚化爐、事業廢棄物焚化爐及醫療廢棄物焚化爐煙道廢氣中總PCDD/Fs I-TEQ排放係數平均值分別為0.750、0.874、3.30及16.7 μg I-TEQ/ton-waste；電弧爐、煉鋼廠SINTER製程、煉焦爐、水泥窯、二次鋁精煉廠及二次銅精煉廠煙道廢氣中總PCDD/Fs I-TEQ排放係數平均值分別為3.64、0.455、0.0134、0.00891、1.40及0.735 μg I-TEQ/ton-feedstock。Y工業區之PCDD/Fs年排放總量為13.1 g I-TEQ/yr，各類污染源佔總貢獻量分別為大型都市垃圾焚化爐(0.885 %)、中小型廢棄物焚化爐(0.0188 %)、事業廢棄物焚化爐(0.114 %)、醫療廢棄物焚化爐(0.215 %)、電弧爐(33.9 %)、煉鋼廠SINTER製程(64.0 %)、煉焦爐(0.197 %)、水泥窯(0.0922 %)、鋁二級冶煉廠(0.162 %)及銅二級冶煉廠(0.409 %)。其中以電弧爐及煉鋼廠SINTER製程之PCDD/Fs年排放總量最高，其總和佔總貢獻量之97.9%。
第一季至第四季周界大氣總I-TEQ濃度平均值分別為0.0765、0.0707、0.132及0.0903 pg I-TEQ/Nm3，由Y工業區第一季至第四季周界大氣採樣點所得濃度之等位軌跡圖，可知位於電弧爐及煉鋼廠SINTER製程等固定污染源下風處周界大氣中PCDD/Fs濃度較高，故推測Y工業區周界大氣中PCDD/Fs濃度受到電弧爐及煉鋼廠SINTER製程等固定污染源之影響。第一季至第四季周界植物總I-TEQ濃度平均值分別為7.85、3.17、5.41及10.6 ng I-TEQ/kg，由Y工業區第一季至第四季周界植物採樣點所得濃度之等位軌跡圖，可知第一季位於電弧爐及煉鋼廠SINTER等固定污染源下風處周界植物中PCDD/Fs濃度較高，故推測第一季採樣當時Y工業區周界植物中PCDD/Fs濃度受到電弧爐及燒結爐等固定污染源之影響。第二季、第三季及第四季整個周界植物PCDD/Fs含量之等位軌跡圖似乎與其他固定污染源之分佈相當密切，H採樣點及J採樣點周邊屬於濃度較高之區域。第一季至第四季周界土壤總I-TEQ濃度平均值分別為6.08、5.78、10.2及11.3 ng I-TEQ/kg，由Y工業區第一季至第四季周界土壤採樣點所得濃度之等位軌跡圖，可知整個周界土壤PCDD/Fs含量之等位軌跡圖似乎與其他固定污染源之分佈相當密切，H採樣點及J採樣點周邊屬於濃度較高之區域。

In order to understand the influences of surrounding environments from PCDD/Fs emission sources in the Y industrial zone, the following PCDD/Fs emission sources were investigated: two large-scale municipal solid waste incinerators (MSWI1 and MSWI2); one small-scale municipal solid waste incinerator (MSWI3); two industrial waste incinerators (IWI1 and IWI2); one medical waste incinerator (MWI); five electric furnaces (EAFs); four sinter planes (SINTERs); one coke oven plane (COKE); one cement kiln (CEMENT); two secondary aluminum smelters (ALS1 and ALS2); and, one secondary copper smelter (COP). By the investigations of these PCDD/Fs in the stack flue gas of emission sources, the overall emission quantity of PCDD/Fs from the Y industrial zone and the congener profiles in the stack flue gas was estimated. Furthermore, we chose ten sampling sites to investigate PCDD/Fs concentrations in ambient air‚ leaves and soil around the Y industrial zone and the non-industrial zone. By the comparisons between the PCDD/Fs concentrations in environmental media and the PCDD/Fs concentrations from PCDD/Fs emission sources using cluster analysis and principal component analysis, the influence of these emission sources on the surrounding environment was assessed.
The concentration means from the stack flue gases were as follows: large-scale MSWIs, 0.0632ng I-TEQ/Nm3; small-scale MSWI, 0.239ng I-TEQ/Nm3; IWIs, 0.145ng I-TEQ/Nm3; MWI, 1.64ng I-TEQ/Nm3; EAFs, 0.477ng I-TEQ/Nm3; SINTERs, 0.326ng I-TEQ/Nm3; COKE, 0.00870ng I-TEQ/Nm3; CEMENT, 0.0138ng I-TEQ/Nm3; ALSs, 0.0504ng I-TEQ/Nm3; and, COP 0.310ng I-TEQ/Nm3.
The emission factors of PCDD/Fs from the stack flue gases were as follows: large-scale MSWIs, 0.750 μg I-TEQ/ton-waste; small-scale MSWI, 0.874 μg I-TEQ/ton-waste; IWIs, 3.30 μg I-TEQ/ton-waste; and MWI, 16.7 μg I-TEQ/ton-waste. The emission factors of PCDD/Fs from the stack flue gases were as follows: EAFs, 3.64 μg I-TEQ/ton-feedstock; SINTERs, 0.455 μg I-TEQ/ton-feedstock; COKE, 0.0134 μg I-TEQ/ton-feedstock; CEMENT, 0.00891 μg I-TEQ/ton-feedstock; ALSs, 1.40 μg I-TEQ/ton-feedstock; and, COP, 0.735 μg I-TEQ/ton-feedstock. The estimated total annual emission of PCDD/Fs from these emission sources in the Y industrial zone was 13.1 g I-TEQ/yr (large-scale MSWIs, 0.885%; small-scale MSWIs, 0.0188%; industrial waste incinerators, 0.114%; medical waste incinerators, 0.215%; electric furnaces, 33.9%; sinter planes, 64.0%; coke oven planes, 0.197%; cement kilns, 0.0922%; secondary aluminum smelters, 0.162%; and secondary copper smelters, 0.409%). The analytical results revealed that the annual emission of PCDD/Fs from metallurgical processes reached a maximum value in the Y industrial zone. The sum of annual emission from EAFs and SINTERs was 97.9%.
The PCDD/Fs average concentrations of ambient air for four seasons around the Y industrial zone were 0.0765, 0.0707, 0.132 and 0.0903 pg I-TEQ/Nm3. The distribution curve of PCDD/Fs concentrations for four seasons indicates that the area downwind of the EAFs and SINTERs had higher PCDD/Fs levels in ambient air. And as a result we concluded that the PCDD/Fs concentrations of ambient air around the Y industrial zone were affected by the EAFs and SINTERs. The PCDD/Fs average concentrations of leaves for four seasons around the Y industrial zone were 7.85, 3.17, 5.41, and 10.6 ng I-TEQ/kg. From the distribution curve of PCDD/Fs concentrations of the first season, we found that the area downwind of the EAFs and SINTERs had higher PCDD/Fs levels in the leaves. And as a result we concluded that the PCDD/Fs concentrations of leaves from the first season around the Y industrial zone were affected by the EAFs and SINTERs. The distribution curve of PCDD/Fs concentrations of leaves from the second, third and fourth seasons seems to be intimate with other pollution sources. The edges of H and J sampling sites had higher PCDD/Fs levels in leaves. The PCDD/Fs average concentrations of soil for four seasons around the Y industrial zone were 6.08, 5.78, 10.2, and 11.3 ng I-TEQ/kg. The distribution curve of PCDD/Fs concentrations for four seasons seems to be intimate with other pollution sources and the edges of H and J sampling sites had higher PCDD/Fs levels in the soil.

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