爲了瞭解Y工業區PCDD/Fs污染源對周遭環境之影響，本研究選定Y工業區中一座大型都市垃圾焚化爐、一座小型都市垃圾焚化爐、一座醫療廢棄物焚化爐、一座煉焦爐、三座煉鋼廠SN製程、五座電弧爐及一座二次鋁精煉廠進行PCDD/Fs排放之研究，藉由煙道廢氣PCDD/Fs之檢測，以建立本土PCDD/Fs排放源之貢獻量及其煙道廢氣特徵剖面，並於Y工業區周界選定數個採樣點進行採樣，調查Y工業區周界環境中各介質（大氣、植物、土壤）之PCDD/Fs含量，藉由本研究中各類污染源之分佈及排放特性，與周界環境中PCDD/Fs 之流佈相比對，亦利用主成分分析及階層集群分析等方法分析，以釐清當地PCDD/Fs污染源污染對周遭環境之影響。研究成過如下：大型都市垃圾焚化爐、小型一般廢棄物焚化爐、醫療廢棄物焚化爐、煉焦爐、煉鋼廠SN製程、電弧爐、二次鋁精煉廠煙道廢氣中總PCDD/Fs I-TEQ濃度平均值分別為0.0917、10.8、0.557、0.0369、1.41、0.196、0.245ng I-TEQ/Nm3； 大型都市垃圾焚化爐、小型一般廢棄物焚化爐、醫療廢棄物焚化爐煙道廢氣中總PCDD/Fs I-TEQ排放係數平均值分別為0.696、26.0、6.95 μg I-TEQ/ton-waste；煉焦爐、煉鋼廠SN製程、電弧爐、二次鋁精煉廠煙道廢氣中總PCDD/Fs I-TEQ排放係數平均值分別為0.155、2.21、1.49、4.29 μg I-TEQ/ton-feedstock。本研究推估所得之Y工業區PCDD/Fs年排放總量為37.98g I-TEQ/yr，其中大型都市垃圾焚化爐、中小型廢棄物焚化爐、醫療廢棄物焚化爐、事業廢棄物焚化爐、煉焦爐、煉鋼廠SN製程、電弧爐、鋁二級冶煉廠、銅二級冶煉廠分別佔總貢獻量之0.848%、0.445%、0.0219%、0.0226、2.60% 、86.1%、6.48%、1.78%、1.71%。其中以煉鋼廠SN製程及電弧爐之PCDD/Fs年排放總量最高，其總和佔總貢獻量之92.6%。Y工業區周界大氣總I-TEQ濃度介於0.0576 ~0.260 pg I-TEQ/Nm3之間，總I-TEQ濃度平均值為0.116 pg I-TEQ/Nm3。Y工業區植物葉片及周界土壤總I-TEQ含量平均值分別為9.49與10.6 ng I-TEQ/kg，周界大氣、植物及土壤中PCDD/Fs含量分佈曲線，皆爲位於電弧爐與煉鋼廠SN製程等固定污染源下風處之含量較高，且依據階層集群與主要成份分析結果顯示大氣之PCDD/Fs特徵剖面與金屬冶煉業之煙道廢氣PCDD/Fs特徵剖面關連性頗高，故推測Y工業區周界大氣、植物及土壤中PCDD/Fs含量受到電弧爐與煉鋼廠SN製程之影響。

　　This study examined the characteristics of polychlorinated dibenzo-p-dioxins and polychlorinated dibenzofurans (PCDD/Fs) in emissions, ambient air‚ leaves and soil at the Y industrial zone. The following PCDD/Fs emmision sources were investigated: one large-scale municipal solid waste incinerator (MSWI1); one small-scale municipal solid waste incinerator (MSWI2); one medical waste incinerator (MWI); one coke oven plane (COKE); three sinter planes (SNs); five electric furnaces (EAFs); and, one secondary aluminum smelter (ALS). The emission factors of PCDD/Fs in the stack flue gases were determined‚ and the overall emission quantity of PCDD/Fs from the Y industrial zone was estimated. Finally, the influence of these emission sources on the surrounding environment was assessed. The concentration means from the stack flue gases were as follows: large-scale MSWI, 0.0917ng I-TEQ/Nm3; small-scale MSWI, 10.8ng I-TEQ/Nm3; MWI, 0.557ng I-TEQ/Nm3; COKE, 0.0369ng I-TEQ/Nm3; SNs, 1.41ng I-TEQ/Nm3; EAFs, 0.196ng I-TEQ/Nm3; and, ALS 0.245ng I-TEQ/Nm3. The emission factors of PCDD/Fs from the stack flue gases were as follows: large-scale MSWI, 0.696 μg I-TEQ/ton-waste; small-scale MSWI, 26.0 μg I-TEQ/ton-waste; and, MWI, 6.95 μg I-TEQ/ton-waste. The emission factors of PCDD/Fs from the stack flue gases were as follows: COKE, 0.155 μg I-TEQ/ton-feedstock; SNs, 2.21 μg I-TEQ/ton-feedstock; EAFs, 1.49 μg I-TEQ/ton-feedstock; and, ALS, 4.29 μg I-TEQ/ton-feedstock. The estimated total annual emission of PCDD/Fs from these emission sources in the Y industrial zone was 37.98 g I-TEQ/yr (large-scale MSWIs, 0.848%; small-scale MSWIs, 0.445%; medical waste incinerators, 0.0219%; industrial waste incinerator, 0.0226%; coke oven planes, 2.60%; sinter planes, 86.1%; electric furnaces, 6.48%; secondary aluminum smelters, 1.78%; secondary copper smelters, 1.71%). The analytical results revealed that the annual emission of PCDD/Fs from metallurgical processes reached a maximum value in the Y industrial zone. The sum of annual emission from SNs and EAFs was 92.6%.

　　The PCDD/Fs concentrations of ambient air around the Y industrial zone ranged from 0.0576~0.260 pg I-TEQ/Nm3 (mean, 0.116 pg I-TEQ/Nm3). The average amount of PCDD/Fs in leaves and soil around the Y industrial zone were, respectively, 9.49 and 10.6 ng I-TEQ/kg. The distribution curve of PCDD/Fs concentrations indicates that the area downwind of the SNs and EAFs had higher PCDD/Fs levels in ambient air, leaves and soil. Furthermore‚ the congener profiles of the stack fule gases of the SNs and EAFs had a strong resemblance to the congener profiles of ambient air. Therefore, the concentrations of PCDD/Fs in ambient air, leaves and soil around the Y industrial zone were significantly influenced by emissions from the SNs and EAFs.

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